搜索结果: 1-10 共查到“化学 classical”相关记录10条 . 查询时间(0.781 秒)
Efficient energy transfer in light-harvesting systems: Quantum-classical comparison, flux network, and robustness analysis
Efficient energy transfer light-harvesting systems Quantum-classical comparison flux network robustness analysis
2014/9/24
Following the calculation of optimal energy transfer in thermal environment in our first paper [J. L. Wu, F. Liu, Y. Shen, J. S. Cao, and R. J. Silbey, New J. Phys.12,105012(2010)],fullquantum dynamic...
Nonadiabatic Dynamics in Open Quantum-Classical Systems: Forward-Backward Trajectory Solution
Nonadiabatic Dynamics Open Quantum-Classical Systems Forward-Backward Trajectory Solution Chemical Physics
2012/5/29
A new approximate solution to the quantum-classical Liouville equation is derived starting from the formal solution of this equation in forward-backward form. The time evolution of a mixed quantum-cla...
Quasi-classical Trajectory Study of C+CD→C2+D at Different Collision Energy
Quasi-classical trajectory Stereodynamics calculation Polarization depen-dent generalized differential cross-section Stereodynamics
2012/4/5
Quasi-classical trajectory calculations have been employed to investigate the influence of collision energy on the stereodynamics of the title reaction C+CD→C2+D on the poten-tial energy surface of th...
SUSTAINING A CONTROVERSY: THE NON-CLASSICAL ION DEBATE
organic chemistry explanation Non-classical Ions controversy
2011/9/7
This paper examines a scientific controversy that raged for twenty years in physical organic chemistry during the second half of the twentieth century. After explaining what was at stake in the Non-Cl...
The influence of dissipation on the quantum-classical correspondence: Stability of stochastic trajectories
dissipation quantum-classical correspondence Stability of stochastic trajectories
2014/9/24
The quantum-classical correspondence in the presence of dissipation is studied. The semiclassical expression for the linear response function of an anharmonic system is expressed in a series containin...
Classical Divergence of Nonlinear Response Functions
Classical Divergence Nonlinear Response Functions
2014/9/24
The time divergence of classical nonlinear response functions reveals the fundamental difficulty of dynamic perturbation based on classical mechanics. The nature of the divergence is established for s...
Quantum-Classical Correspondence in Response Theory
Quantum-Classical Correspondence Response Theory
2014/9/24
The correspondence principle between the quantum commutator^A;^ B and the classical Poisson brackets@fA; Bg is examined in the context of response theory. The classical response function is obtaine...
Nondivergent classical response functions from uncertainty principle: Quasiperiodic systems
Nondivergent classical response functions uncertainty principle Quasi Periodic systems
2014/9/24
Time-divergence in linear and nonlinear classical response functions can be removed by taking a phase-space average within the quantized uncertainty volume O(\
n) around the microcanonical energy sur...
The reorientational relaxation of molecular systems is important in many phenomenon and applications. In this paper, we explore the reorientational relaxation of a model Brownian rotor lattice system ...
Linear and nonlinear response functions of the Morse oscillator: Classical divergence and the uncertainty principle
Linear and nonlinear response functions the Morse oscillator Classical divergence the uncertainty principle
2014/9/24
The algebraic structure of the quantum Morse oscillator is explored to formulate the coherent state,the phase-space representations of the annihilation and creation operators, and their classical limi...