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In this paper, we discuss a strategy for reducing a complex single molecule kinetic process to a set of generic structures (motifs) that are building blocks for a general kinetic scheme. In general, t...
As discussed in the companion paper@J. B. Witkoskie and J. S. Cao, J. Chem. Phys.121, 6361~2004!, preceding paper#, quantitative extraction of information from single molecule experiments by several p...
Single molecule experiments reveal intriguing phenomenon in chemical and biological systems.Several indicators of complex dynamics, including ‘‘intensity’’ correlations, ‘‘event’’ correlations,and cha...
Statistics and correlations of single-molecule sequences of modulated reactions are explicitly evaluated in the stochastic rate representation. The memory function, introduced through the Gaussian app...
The relationship between event-averaged measurements and ensemble averaged measurements can be clarified by averaging along single-molecule trajectories. As a result, phenomenological chemical kinetic...
A modulated N-conformational-channel reactive system is used to model the recent single-molecule enzymatic experiw .x ment Science 282 1998 1877 . Kinetic analysis of the model system clearly demonst...

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